YANG Ji-tao, CHEN Lin-xia, WANG Gang-gang, LIU Jie, YANG Min. Study on adsorption of tetracycline by magnetic microsphere crosslinked with TG,Pepsin and Papain[J]. Science and Technology of Food Industry, 2016, (24): 226-232. DOI: 10.13386/j.issn1002-0306.2016.24.035
Citation: YANG Ji-tao, CHEN Lin-xia, WANG Gang-gang, LIU Jie, YANG Min. Study on adsorption of tetracycline by magnetic microsphere crosslinked with TG,Pepsin and Papain[J]. Science and Technology of Food Industry, 2016, (24): 226-232. DOI: 10.13386/j.issn1002-0306.2016.24.035

Study on adsorption of tetracycline by magnetic microsphere crosslinked with TG,Pepsin and Papain

More Information
  • Received Date: June 29, 2016
  • Different enzyme- immobilized magnetic adsorbents were prepared by using glutaraldehyde to crosslink TG,Pepsin and Papain on amination magnetic microspheres. The adsorbents structure characteristics were analyzed by scanning electron microscope and infrared spectroscopy.The effect of initial concentration,adsorbent temperature,time and acidity on the adsorption of tetracycline in aqueous solution was investigated. Experimental results showed that the static adsorption accorded with the Pseudo- second- order kinetic and Freundlich adsorption isotherm,adsorption mechanism was not only multilayer chemical adsorption process but also endothermic process.Under the same adsorption temperature,the adsorption rate of order was Pepsin- AMM >Papain- AMM > TG- AMM. In the adsorption temperature was 318 K,adsorption process was spontaneous,the maximum adsorption capacities were 99.72,64.97 and 67.52 mg / g.
  • [1]
    S A Sassman,L S Lee.Sorption of Three Tetracyclines by Several Soils:Assessing the Role of p H and Cation Exchange[J].Environmental Science&Technology,2005,39(19):7452-7459.
    [2]
    Holmstrm K,Grslund S,Wahlstrm A,et al.Antibiotic use in shrimp farming and implications for environmental impacts and human health[J].International Journal of Food Science&Technology,2003,38(3):255-266.
    [3]
    邵一如,席北斗,曹金玲,等.抗生素在城市污水处理系统中的分布及去除[J].环境科学与技术,2013(7):85-92.
    [4]
    周启星,罗义,王美娥.抗生素的环境残留、生态毒性及抗性基因污染[J].生态毒理学报,2007,2(3):243-251.
    [5]
    王健,贲伟伟,强志民,等.我国养猪业废弃物中四环素类、磺胺类抗生素及相关抗性基因污染研究进展[J].生态毒理学报,2015,10(5):2-10.
    [6]
    张大文,王冬根,胡丽芳,等.猪肉产品中四环素类药物残留风险评估[J].农产品质量与安全,2014(6):34-37.
    [7]
    中华人民共和国卫生部.GB/T 5009.116-2003畜、禽肉中土霉素、四环素、金霉素和强力霉素残留量的测定(高效液相色谱法)[S].北京:中国标准出版社,2003.
    [8]
    袁冬梅,李一婧.养殖水产品中四环素类抗生素残留的高效液相色谱测定法[J].食品工业科技,2008(1):281-281.
    [9]
    Chen K,Geng S,Huang J K,et al.Editorial for the special issue on food safety in China[J].Journal of Integrative Agriculture,2015,14(11):2135.
    [10]
    Mojtaba Hedayati Marzbali,Mohamad Esmaieli,Hossein Abolghasemi,et al.Tetracycline adsorption by H3PO4-activated carbon produced from apricot nut shells:A batch study[J].Process Safety and Environmental Protection,2016.
    [11]
    Martins A C,Pezoti O,Cazetta A L,et al.Removal of tetracycline by Na OH-activated carbon produced from macadamia nut shells:Kinetic and equilibrium studies[J].Chemical Engineering Journal,2015,260:291-299.
    [12]
    李钢.鸢尾活性炭的制备及对四环素和Ni(Ⅱ)吸附特性的研究[D].济南:山东大学,2014.
    [13]
    刘江国,李杰霞,陈玉成,等.改性玉米秸秆对四环素废水的吸附研究[J].环保科技,2009,15(4):27-30.
    [14]
    Jin K,Liu H,Zheng Y M,et al.Systematic study of synergistic and antagonistic effects on adsorption of tetracycline and copper onto a chitosan[J].Journal of Colloid&Interface Science,2010,344(1):117-125.
    [15]
    粟顺兴,雷俊茹,张中杰.磁性酵母茵微球体的制备及吸附四环素的研究[J].应用化工,2012(12):2099-2102.
    [16]
    刘希,张宇峰,罗平.改性花生壳对四环素类抗生素的吸附特性研究[J].环境污染与防治,2013,35(5):35-39.
    [17]
    Yang C,Wu J,Hou Y.Fe3O4nanostructures:synthesis,growth mechanism,properties and applications.[J].Chemical Communications,2011,47(18):5130-41.
    [18]
    侯鉴璇.磁性材料的制备及其在固定化酶方面的应用[D].北京:北京化工大学,2014.
    [19]
    王冰,王云普,曾家豫,等.沙蒿胶磁性微球固定化脂肪酶及部分理化性质的研究[J].食品工业科技,2008(1):143-145.
    [20]
    张春红.食品酶制剂及应用[M].北京:中国计量出版社,2008:150-240.
    [21]
    吴文兵,杨婉身,王显祥.氨基磁性微球固定化木瓜蛋白酶及其应用[J].生物技术,2010,20(5):78-81.
    [22]
    周冉,常明,王飞,等.仿生硅化-磁性Fe3O4固定化木瓜蛋白酶的性质[J].食品工业科技,2014,35(12):180-183.
    [23]
    赵良忠,刘静霆,任光云,等.磁性壳聚糖微球固定化胃蛋白酶的研究[J].食品科学,2008,29(11):316-323.
    [24]
    Chao Y,Zhu W,Chen F,et al.Commercial Diatomite for Adsorption of Tetracycline Antibiotic from Aqueous Solution[J].Separation Science&Technology,2014,49(14):2221-2227.
    [25]
    王建芝.功能化磁性纳米材料的制备及其固定化酶的研究[D].甘肃:兰州大学,2015.
    [26]
    Brigante M,Schulz P C.Remotion of the antibiotic tetracycline by titania and titania-silica composed materials[J].Journal of Hazardous Materials,2011,192(3):1597-608.
    [27]
    近藤精一.吸附科学[M].北京:化学工业版社,2006:10-200.
    [28]
    Adriano W S,Veredas V,Santana C C,et al.Adsorption of amoxicillin on chitosan beads:Kinetics,equilibrium and validation of finite bath models[J].Biochemical Engineering Journal,2006,27(2):132-137.
    [29]
    Chang P H,Li Z,Yu T L,et al.Sorptive removal of tetracycline from water by palygorskite[J].Journal of Hazardous Materials,2009,165(1-3):148-155.
    [30]
    王雅群,潘道东.磁性分子印迹固相萃取食品中的四环素类抗生素残留[J].食品工业科技,2015,36(18):53-58.
  • Related Articles

    [1]LI Xinzhi, LIU Xi, XU Xinyu, ZHOU Qiyang, WU Changzheng, TONG Xing, OU Shiyi. Effect of Gradient Heating Method on the Microbial Changes and Flavor Formation of Liquid-State Soy Sauce Fermented with Different Salt Concentrations[J]. Science and Technology of Food Industry, 2024, 45(9): 106-114. DOI: 10.13386/j.issn1002-0306.2023080043
    [2]WANG Bei, YU Junjuan. Effects of Sterilization Technology and Storage Temperature on the Quality of Fermented Puffer Fish Sauce during the Preservation[J]. Science and Technology of Food Industry, 2024, 45(7): 313-319. DOI: 10.13386/j.issn1002-0306.2023050103
    [3]MA Yi, XIE Liming, XIAO Xiongjun, YU Kangjie, WEI Ziyun, XIONG Rong, YU Xiao, HUANG Huiling. Effect of Fermentation Temperature on the Quality of Pear Wine[J]. Science and Technology of Food Industry, 2023, 44(11): 336-342. DOI: 10.13386/j.issn1002-0306.2022110057
    [4]XU Wei, MA Ting-ting, LI Jia-mei, MA Zhi-yu, CHAI Li-na. Effect of Fermentation Time on the Formation of Organic Acid and Its Acidity in Russian Bread Dough[J]. Science and Technology of Food Industry, 2019, 40(22): 82-86,92. DOI: 10.13386/j.issn1002-0306.2019.22.015
    [5]DING Xi, TANG Shan-hu, LI Si-ning, MO Ran, XIAO Ting. Effects of Constant Fermentation Temperatures on Physicochemical Properties of Fermented Yak Meat Sausage[J]. Science and Technology of Food Industry, 2019, 40(5): 42-47. DOI: 10.13386/j.issn1002-0306.2019.05.008
    [6]WU Yu-xin, ZHANG Ke-xin, JIANG Hui, TANG Xiao-juan, XU Yan, HUANG Wei-ning, LI Ning, Filip Arnaut. Research on Ultrastructure of Dough and Aroma Characteristics of Bread Containing Glutinous Rice Fermented at Different Fermentation Time[J]. Science and Technology of Food Industry, 2019, 40(2): 29-36. DOI: 10.13386/j.issn1002-0306.2019.02.006
    [7]ZHAO Xin, WANG Qiang. Study on comparisons of different ripening fermentation periods fermented Shuidouchi in their physicochemical properties[J]. Science and Technology of Food Industry, 2014, (11): 346-349. DOI: 10.13386/j.issn1002-0306.2014.11.068
    [8]WANG Xiao-nan, LIN Li-jie, WANG Feng-jun. Optimization of fermentation conditions for preparing walnut soy sauce[J]. Science and Technology of Food Industry, 2014, (05): 209-212. DOI: 10.13386/j.issn1002-0306.2014.05.040
    [9]YIN Wen-ying, CUI Chun, CHEN Ling, LIN Zong-yi, ZHAO Mou-ming. Effects of fermentation temperature on the quality of soy sauce[J]. Science and Technology of Food Industry, 2014, (02): 154-157. DOI: 10.13386/j.issn1002-0306.2014.02.085
    [10]发酵法桑汁饮料加工工艺的研究[J]. Science and Technology of Food Industry, 1999, (05): 35-37. DOI: 10.13386/j.issn1002-0306.1999.05.012
  • Cited by

    Periodical cited type(14)

    1. 刘非凡,温纪平,展小彬,石松业,李柯新,唐浩洁. 冷等离子体处理在食品中的应用研究进展. 食品研究与开发. 2024(12): 181-188 .
    2. 闵照永. 等离子体活化水及微波协同处理对鲜湿面片特性的影响. 食品科技. 2024(06): 180-186 .
    3. 高婷,尹凯静,邵栋梁,赵丹丹,戴文娜. 低温等离子体技术杀灭食源性致病菌的研究进展. 农产品加工. 2024(14): 100-103 .
    4. 方镇洲,杨体园,赵玲艳,邓洁红. 低温等离子体处理对华容大叶芥菜贮藏品质的影响. 食品安全质量检测学报. 2024(20): 257-262 .
    5. 张腾,江昊. 超声渗透等离子活化水对香蕉切片鲜切品质的影响. 包装工程. 2023(05): 65-74 .
    6. 萧文宇,吴迅,黄显斌,李玲,何志平,郭俭. 低温等离子体活化水对蓝莓表面微生物抑制作用及其贮藏品质的影响. 食品工业科技. 2023(08): 359-365 . 本站查看
    7. 颜心怡,李锦晶,李赤翎,吴金鸿,俞健,王发祥,刘永乐,李向红. 冷等离子体技术对食品组分的影响及其作用机制. 食品工业科技. 2023(12): 445-454 . 本站查看
    8. 李芮,宋雅琪,周丹丹,屠康. 等离子体活化水对鲜切莲藕杀菌及保鲜的影响. 食品与生物技术学报. 2023(10): 30-40 .
    9. 田方,徐咏菁,孙志栋,周琦,王志远,华镇南,蔡路昀. 低温等离子体处理对鲜切猕猴桃片微观结构及理化特性的影响. 食品与发酵工业. 2023(21): 167-174 .
    10. 赵莹,严龙飞,严文静,章建浩. 低温等离子体活化水与介质阻挡放电联合处理对草莓冷杀菌效果及品质的影响. 食品科学. 2022(17): 105-116 .
    11. 韩扬,朱成志,李沁雨,李立,马新新,赵志军,包怡红. ε-聚赖氨酸复合保鲜剂对鸡毛菜品质及微生物的影响. 食品与发酵工业. 2022(18): 205-212 .
    12. 白亚龙,廖小艳,崔妍. 消除鲜食生菜中细菌污染的研究进展. 食品科学. 2022(19): 367-374 .
    13. 相启森,张嵘,杜桂红,王利敏,蒋爱民. 等离子体活化水对沙门氏菌的灭活作用及机制研究. 食品工业科技. 2021(08): 138-143 . 本站查看
    14. 翟娅菲,田佳丽,相启森,禹晓,申瑞玲,王章存. 非热加工技术在果蔬保鲜中的应用. 食品工业. 2021(05): 327-332 .

    Other cited types(9)

Catalog

    Article Metrics

    Article views (145) PDF downloads (72) Cited by(23)

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return